Surrogate Model Assisted Design of Silicon Anode Considering Lithiation Induced Stresses


Zheng Z., Chen B., Gurumukhi Y., Cook J., ATEŞ M. N., Miljkovic N., ...Daha Fazla

2019 IEEE International Reliability Physics Symposium, IRPS 2019, California, Amerika Birleşik Devletleri, 31 Mart - 04 Nisan 2019, cilt.2019-March, (Tam Metin Bildiri) identifier

  • Yayın Türü: Bildiri / Tam Metin Bildiri
  • Cilt numarası: 2019-March
  • Doi Numarası: 10.1109/irps.2019.8720601
  • Basıldığı Şehir: California
  • Basıldığı Ülke: Amerika Birleşik Devletleri
  • Anahtar Kelimeler: GP based surrogate model, Lithiation induced stress, Multiphysics modeling, Silicon anode
  • Boğaziçi Üniversitesi Adresli: Hayır

Özet

Silicon-based lithium ion battery anodes are attracting considerable attention due to their high theoretical capacity. However, the significant volume change of silicon during lithiation/de-lithiation cycles restricts its application. A novel bi-continuous Si anode, designed to mitigate the effect of cycling-induced volume changes, is investigated in this study. The effects of the design parameters and the operating conditions of the anode are explored via multi-physics simulation model. It is found that, with the novel anode structure, battery charging C rate has little impact on the mechanical properties. However, the anode structural design parameters would largely influence the stress distribution on the anode. Thus, a Gaussian Processes (GP) based surrogate model is developed to assist the design optimization of the Si anode, while using the simulated results from a multiphysics simulation model as training data. An optimized Si anode design can then be extracted efficiently based upon the developed surrogate model.